黃河三角洲土壤和水體沉積物中典型有機(jī)污染物的環(huán)境行為研究
發(fā)布時(shí)間：2020-12-07 10:21
本論文以黃河三角洲自然保護(hù)區(qū)所采集的土壤樣品、黃河入海口所采集的表層沉積物樣品以及老黃河入�？谒杉某练e柱樣品為研究對(duì)象,通過(guò)索氏抽提、微波萃取、超聲提取、氣相色譜質(zhì)譜分析以及同位素定年等實(shí)驗(yàn)分析方法以及比值分析、相關(guān)性分析、因子分析和聚類分析等數(shù)據(jù)處理方法,對(duì)多環(huán)芳烴、多氯聯(lián)苯以及多溴聯(lián)苯醚這三種典型有機(jī)污染物在黃河三角洲土壤和水體沉積物中的賦存特征、空間分布、輸入途徑以及潛在風(fēng)險(xiǎn)進(jìn)行了研究。通過(guò)研究主要取得了如下結(jié)果：(1)多環(huán)芳烴、多氯聯(lián)苯和多溴聯(lián)苯醚在黃河三角洲土壤和水體沉積物中分布廣泛,但與國(guó)內(nèi)外其它地區(qū)相比,本研究區(qū)域有機(jī)物污染水平相對(duì)較低；老黃河入海口沉積柱中多環(huán)芳烴含量的歷史變化趨勢(shì)有效地記錄了20世紀(jì)60年代以來(lái)該地區(qū)的人類活動(dòng)以及我國(guó)經(jīng)濟(jì)發(fā)展中的重要事件；(2)有機(jī)碳并不總是影響該地區(qū)有機(jī)污染物分布的主要因素：有機(jī)碳與多環(huán)芳烴在該地區(qū)呈現(xiàn)顯著的相關(guān)性,但多氯聯(lián)苯和多溴聯(lián)苯醚與有機(jī)碳間的相關(guān)性較弱；(3)該地區(qū)多環(huán)芳烴的主要輸入途徑有石油、煤、生物質(zhì)、天然氣以及機(jī)動(dòng)車尾氣的排放,而多氯聯(lián)苯和多溴聯(lián)苯醚的來(lái)源主要和過(guò)去對(duì)多氯聯(lián)苯、多溴聯(lián)苯醚商品的生產(chǎn)使用以及高溴代多溴...
【文章來(lái)源】：中國(guó)科學(xué)技術(shù)大學(xué)安徽省 211工程院校 985工程院校
【文章頁(yè)數(shù)】：229 頁(yè)
【學(xué)位級(jí)別】：博士
【部分圖文】：
圖.娜七.自.
【參考文獻(xiàn)】：
期刊論文
[1]Polybrominated diphenyl ethers in soil from three typical industrial areas in Beijing, China[J]. Yongfei Zhang,Shan Fu,Xinchun Liu,Zheng Li,Yuan Dong. Journal of Environmental Sciences. 2013(12)
[2]Topsoil dichlorodiphenyltrichloroethane and polychlorinated biphenyl concentrations and sources along an urban-rural gradient in the Yellow River Delta[J]. Wenjun Xie 1,Aiping Chen 2,Jianyong Li 3,Qing Liu 1,Hongjun Yang 1,Tao Wu 1,Zhaohua Lu 1,2,1.Shandong Key Laboratory of Eco-Environmental Science for the Yellow River Delta,Binzhou University,Binzhou 256603,China. 2.Institute of Restoration Ecology,China University of Mining and Technology,Beijing 100083,China 3.Jinan Entry-Exit Inspection and Quarantine Bureau,Jinan 250000,China. Journal of Environmental Sciences. 2012(09)
[3]Sedimentary record of polycyclic aromatic hydrocarbons in Lake Erhai,Southwest China[J]. Jianyang Guo 1,Zhang Liang 1,2,Haiqing Liao 2,Zhi Tang 2,Xiaoli Zhao 2,Fengchang Wu 2,1.State Key Laboratory of Environmental Geochemistry,Institute of Geochemistry,Chinese Academy of Sciences,Guiyang 550002,China.2.State Environmental Protection Key Laboratory for Lake Pollution Control,Research Center of Lake Eco-Environment,Chinese Research Academy of Environmental Sciences,Beijing 100012,China. Journal of Environmental Sciences. 2011(08)
[4]Distribution of polybrominated diphenyl ethers and decabromodiphenylethane in surface sediments from Fuhe River and Baiyangdian Lake,North China[J]. Guocheng Hu 1,2,Zhencheng Xu 1,Jiayin Dai 2,Bixian Mai 3,Hong Cao 2,Jianshe Wang 2,Zhimin Shi 2,Muqi Xu 2,1.Metropolitan Environment Center,South China Institute of Environmental Sciences,Ministry of Environmental Protection,Guangzhou 510655,China.2.Key Laboratory of Animal Ecology and Conservation Biology,Institute of Zoology,Chinese Academy of Sciences,Beijing 100101,China 3.State Key Laboratory of Organic Chemistry,Guangzhou Institute of Geochemistry,Chinese Academy of Sciences,Guangzhou 510640,China. Journal of Environmental Sciences. 2010(12)
[5]Distribution of polycyclic aromatic hydrocarbons in sediments from Yellow River Estuary and Yangtze River Estuary,China[J]. HUI Yamei1, ZHENG Minghui1, LIU Zhengtao2, GAO Lirong1 1. State Key Laboratory of Environmental Chemistry and Ecotoxicology, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China. 2. China Research Academy of Environmental Sciences, Beijing 100012, China. Journal of Environmental Sciences. 2009(12)
[6]黃河三角洲自然保護(hù)區(qū)丹頂鶴生境適宜性變化分析(英文)[J]. 曹銘昌,劉高煥. Journal of Forestry Research. 2008(02)
[7]現(xiàn)代黃河三角洲土壤中多氯聯(lián)苯來(lái)源解析研究[J]. 劉靜,崔兆杰,范國(guó)蘭,許宏宇. 環(huán)境科學(xué). 2007(12)
[8]Chronology of Holocene lacustrine sediments in Co Ngoin, central Tibetan Plateau[J]. WU Yanhong1, WANG Sumin1& HOU Xinhua1,3 1. Key Laboratory of Lake Sedimentation and Environment, Nanjing Institute of Geography and Limnology, Chinese Academy of Sciences, Nanjing 210008, China; 2. Institute of Tibetan Plateau Research, Chinese Academy of Sciences, Beijing 10085, China; 3. Graduate University of Chinese Academy of Sciences, Beijing 100039, China. Science in China(Series D:Earth Sciences). 2006(09)
[9]多環(huán)芳烴的光致毒效應(yīng)[J]. 孫紅文,李書霞. 環(huán)境科學(xué)進(jìn)展. 1998(06)
博士論文
[1]溴代阻燃劑的分析方法及其在黃河三角洲土壤中的污染特征[D]. 苑金鵬.山東大學(xué) 2013
本文編號(hào)：2903083
【文章來(lái)源】：中國(guó)科學(xué)技術(shù)大學(xué)安徽省 211工程院校 985工程院校
【文章頁(yè)數(shù)】：229 頁(yè)
【學(xué)位級(jí)別】：博士
【部分圖文】：
圖.娜七.自.
【參考文獻(xiàn)】：
期刊論文
[1]Polybrominated diphenyl ethers in soil from three typical industrial areas in Beijing, China[J]. Yongfei Zhang,Shan Fu,Xinchun Liu,Zheng Li,Yuan Dong. Journal of Environmental Sciences. 2013(12)
[2]Topsoil dichlorodiphenyltrichloroethane and polychlorinated biphenyl concentrations and sources along an urban-rural gradient in the Yellow River Delta[J]. Wenjun Xie 1,Aiping Chen 2,Jianyong Li 3,Qing Liu 1,Hongjun Yang 1,Tao Wu 1,Zhaohua Lu 1,2,1.Shandong Key Laboratory of Eco-Environmental Science for the Yellow River Delta,Binzhou University,Binzhou 256603,China. 2.Institute of Restoration Ecology,China University of Mining and Technology,Beijing 100083,China 3.Jinan Entry-Exit Inspection and Quarantine Bureau,Jinan 250000,China. Journal of Environmental Sciences. 2012(09)
[3]Sedimentary record of polycyclic aromatic hydrocarbons in Lake Erhai,Southwest China[J]. Jianyang Guo 1,Zhang Liang 1,2,Haiqing Liao 2,Zhi Tang 2,Xiaoli Zhao 2,Fengchang Wu 2,1.State Key Laboratory of Environmental Geochemistry,Institute of Geochemistry,Chinese Academy of Sciences,Guiyang 550002,China.2.State Environmental Protection Key Laboratory for Lake Pollution Control,Research Center of Lake Eco-Environment,Chinese Research Academy of Environmental Sciences,Beijing 100012,China. Journal of Environmental Sciences. 2011(08)
[4]Distribution of polybrominated diphenyl ethers and decabromodiphenylethane in surface sediments from Fuhe River and Baiyangdian Lake,North China[J]. Guocheng Hu 1,2,Zhencheng Xu 1,Jiayin Dai 2,Bixian Mai 3,Hong Cao 2,Jianshe Wang 2,Zhimin Shi 2,Muqi Xu 2,1.Metropolitan Environment Center,South China Institute of Environmental Sciences,Ministry of Environmental Protection,Guangzhou 510655,China.2.Key Laboratory of Animal Ecology and Conservation Biology,Institute of Zoology,Chinese Academy of Sciences,Beijing 100101,China 3.State Key Laboratory of Organic Chemistry,Guangzhou Institute of Geochemistry,Chinese Academy of Sciences,Guangzhou 510640,China. Journal of Environmental Sciences. 2010(12)
[5]Distribution of polycyclic aromatic hydrocarbons in sediments from Yellow River Estuary and Yangtze River Estuary,China[J]. HUI Yamei1, ZHENG Minghui1, LIU Zhengtao2, GAO Lirong1 1. State Key Laboratory of Environmental Chemistry and Ecotoxicology, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China. 2. China Research Academy of Environmental Sciences, Beijing 100012, China. Journal of Environmental Sciences. 2009(12)
[6]黃河三角洲自然保護(hù)區(qū)丹頂鶴生境適宜性變化分析(英文)[J]. 曹銘昌,劉高煥. Journal of Forestry Research. 2008(02)
[7]現(xiàn)代黃河三角洲土壤中多氯聯(lián)苯來(lái)源解析研究[J]. 劉靜,崔兆杰,范國(guó)蘭,許宏宇. 環(huán)境科學(xué). 2007(12)
[8]Chronology of Holocene lacustrine sediments in Co Ngoin, central Tibetan Plateau[J]. WU Yanhong1, WANG Sumin1& HOU Xinhua1,3 1. Key Laboratory of Lake Sedimentation and Environment, Nanjing Institute of Geography and Limnology, Chinese Academy of Sciences, Nanjing 210008, China; 2. Institute of Tibetan Plateau Research, Chinese Academy of Sciences, Beijing 10085, China; 3. Graduate University of Chinese Academy of Sciences, Beijing 100039, China. Science in China(Series D:Earth Sciences). 2006(09)
[9]多環(huán)芳烴的光致毒效應(yīng)[J]. 孫紅文,李書霞. 環(huán)境科學(xué)進(jìn)展. 1998(06)
博士論文
[1]溴代阻燃劑的分析方法及其在黃河三角洲土壤中的污染特征[D]. 苑金鵬.山東大學(xué) 2013
本文編號(hào)：2903083
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